Interplay of Spin and Lattice Degrees of Freedom in the Frustrated Antiferromagnet CdCr₂O₄: High-field and Temperature Induced Anomalies of the Elastic Constants

الأصل · EN

Temperature and magnetic field studies of the elastic constants of the chromium spinel CdCr₂O₄ show pronounced anomalies related to strong spin-phonon coupling in this frustrated antiferromagnet. A detailed comparison of the longitudinal acoustic mode propagating along the [111] direction with theory based on an exchange-striction mechanism leads to an estimate of the strength of the magneto-elastic interaction. The derived spin-phonon coupling constant is in good agreement with previous determinations based on infrared absorption. Further insight is gained from intermediate and high magnetic field experiments in the field regime of the magnetization plateau. The role of the antisymmetric Dzyaloshinskii-Moriya interaction discussed and we compare the spin-phonon coupling in CdCr₂O₄ in both the ordered and disordered states.