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arXiv 2011-06-15 DOI 10.1088/1367-2630/13/5/053059 0 views

Depth dependence of itinerant character in Mn-substituted Sr3Ru2O7

Panaccione, G · Manju, U · Offi, F · Annese, E · Vobornik, I · Torelli, P · Zhu, Z H · Hossain, M A · Simonelli, L · Fondacaro, A · Lacovig, P · Guarino, A · Yoshida, Y · Sawatzky, G A · Damascelli, A

Original · EN

We present a core-level photoemission study of Sr3(Ru 1-xMnx)2O7, in which we monitor the evolution of the Ru-3d fine structure versus Mn substitution and probing depth. In both Ru 3d3/2 and 3d5/2 core levels we observe a clear suppression of the metallic features, i.e. the screened peaks, implying a sharp transition from itinerant to localized character already at low Mn concentrations. The comparison between soft and hard x-ray photoemission, which provides tunable depth sensitivity, reveals that the degree of localized/metallic character for Ru is different at the surface than in the bulk.

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