Calculation of transition probabilities and ac Stark shifts in two-photon laser transitions of antiprotonic helium

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Numerical ab initio variational calculations of the transition probabilities and ac Stark shifts in two-photon transitions of antiprotonic helium atoms driven by two counter-propagating laser beams are presented. We found that sub-Doppler spectroscopy is in principle possible by exciting transitions of the type (n,L)->(n-2,L-2) between antiprotonic states of principal and angular momentum quantum numbers n L-1 35, first by using highly monochromatic, nanosecond laser beams of intensities 10⁴-10⁵ W/cm², and then by tuning the virtual intermediate state close (e.g., within 10-20 GHz) to the real state (n-1,L-1) to enhance the nonlinear transition probability. We expect that ac Stark shifts of a few MHz or more will become an important source of systematic error at fractional precisions of better than a few parts in 10⁹. These shifts can in principle be minimized and even canceled by selecting an optimum combination of laser intensities and frequencies. We simulated the resonance profiles of some two-photon transitions in the regions n=30-40 of the p⁴He+ and p ³He+ isotopes to find the best conditions that would allow this.