Robust antiferromagnetism preventing superconductivity in pressurized Ba0.61K0.39Mn2Bi2

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Here, we report that K-doped BaMn2Bi2 shows no experimental evidence of superconductivity down to 1.5 K under pressures up to 35.6 GPa, however, a tetragonal to an orthorhombic phase transition is observed at pressure of 20 GPa. Theoretical calculations for the tetragonal and orthorhombic phases, on basis of our high-pressure XRD data, find that the AFM order is robust in both of the phases in pressurized Ba0.61K0.39Mn2Bi2. Our experimental and theoretical results suggest that the K-doped BaMn2Bi2 belongs to a strong Hunds AFM metal with a hybridization of localized spin electrons and itinerant electrons, and that its robust AFM order essentially prevents the emergence of superconductivity.