Photon Counting Statistics for Single Molecule Spectroscopy
Barkai, Eli · Jung, YounJoon · Silbey, Robert
Original · EN
We present a general relation between Mandel's Q parameter describing variance of number of photons emitted from a single molecule and a three time correlation function describing a spectral diffusion process the molecule is undergoing. For a prototype of such a stochastic process an exact solution is found which exhibits rich types of physical behaviors.
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