Weak charge-lattice coupling requires reinterpretation of stripes of charge order in La1-xCaxMnO3
Loudon, J. C. · Cox, S. · Williams, A. J. · Attfield, J. P. · Littlewood, P. B. · Midgley, P. A. · Mathur, N. D.
Original · EN
Modulations in manganites attributed to stripes of charge/orbital/spin order are thought to result from strong electron-lattice interactions that lock the superlattice and parent lattice periodicities. Surprisingly in La1-xCaxMnO3(x>0.5, 90 K), convergent beam (3.6 nm spot) electron diffraction patterns rule out charge stacking faults and indicate a superlattice with uniform periodicity. Moreover, large area electron diffraction peaks are sharper than simulations with stacking faults. Since the electron-lattice coupling does not lock the two periodicities (to yield stripes) it may be too weak to strongly localise charge.
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