Spin-enhanced magnetocaloric effect in molecular nanomagnets
Evangelisti, Marco · Candini, Andrea · Ghirri, Alberto · Affronte, Marco · Brechin, Euan K. · McInnes, Eric J. L.
Original · EN
An unusually large magnetocaloric effect for the temperature region below 10 K is found for the Fe14 molecular nanomagnet. This is to large extent caused by its extremely large spin S ground-state combined with an excess of entropy arising from the presence of low-lying excited S states. We also show that the highly symmetric Fe14 cluster core, resulting in small cluster magnetic anisotropy, enables the occurrence of long-range antiferromagnetic order below Tₙ=1.87 K.
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