Electron dynamics in the carbon atom induced by spin-orbit interaction
Rey, H. F. · van der Hart, H. W.
الأصل · EN
We use R-Matrix theory with Time dependence (RMT) to investigate multiphoton ionization of ground-state atomic carbon with initial orbital magnetic quantum number Mₗ=0 and Mₗ=1 at a laser wavelength of 390 nm and peak intensity of 10¹⁴ W cm⁻². Significant differences in ionization yield and ejected-electron momentum distribution are observed between the two values for Mₗ. We use our theoretical results to model how the spin-orbit interaction affects electron emission along the laser polarization axis. Under the assumption that an initial C atom is prepared at zero time delay with Mₗ=0, the dynamics with respect to time delay of an ionizing probe pulse modelled using RMT theory is found to be in good agreement with available experimental data.
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